We report on experimental and simulation-based results using (In, Ga)N alloy quantum barriers in c-plane green light-emitting diode (LED) structures as a means to improve vertical carrier transport and reduce forward voltage (V F). Three-dimensional device simulations that include random alloy fluctuations are used to understand carrier behavior in a disordered potential. The simulated current density-voltage (J-V) characteristics and modified electron-hole overlap |F mod | 2 indicate that increasing the indium fraction in the (In, Ga)N quantum barriers leads to a reduced polarization discontinuity at the interface between the quantum barrier and quantum well, thereby reducing V F and improving |F mod | 2. Maps of electron and hole current ...